InthishapterIstudiedtheinterationofaBose-Einsteinondensateandasingle-mode
optialavity in afull quantum model. In the weak ouplinglimit,the avity mode
ap-points a single ondensate exitationmode that dominantly ouples to the avity eld.
Keepingonlythissingleexitationmode,theBEC-avitysystembeomesformally
anal-ogoustoalass ofopto-mehanialsystems.Byeliminatingthe photoneld,I derived a
quantum master equationfor the BECexitation mode playing the role of the
mehan-ial osillator. Adiabati eliminationof the eld led to an eetive optial potential in
the master equation that has been showed to produe optial bistability.Dissipation of
the avity eld istaken intoaount by diusion and frition terms, with frition being
determinedasthe rst orderorretion totheadiabatieliminationinthe small
param-eter
ω R /κ
.Linearization ofthe master equationestablishes a onnetionwith linearizedmodels desribing vibrating mirrors in the literature, and it enabledus toalulate
an-alytiallyan equilibriumexitation number in the extra weak ouplinglimit.Using the
eetivemasterequation,Isimulatedthenonlinear quantum dynamisofthe BEC
exi-tationinthebistabilityregime.Igenerallyshowedthatquantumtunnelingishinderedby
the dephasing proess aompaniedby photonloss. Nevertheless, oherent matterwave
osillationsarepossible,wherediusionislessdominantforlargeramplitudeosillations.
Dipole-dipole instability of atom louds
in a far-detuned optial dipole trap
Inthis hapter,I onsider theradiativeinteration between oldatoms trapped inside a
far-o-resonanedipoletrap(FORT).Althoughthisworkissomewhatlateraltothemain
bodyoftheThesis,itprovidesaomplementtothemodelsusedintheprevioushapters,
sine it allows for treating an eet whih is usually omittedfrom the desription. The
light-indued dipole-dipole interation between the atoms in a laser eld has indeed
a small eet at typial atom densities and laser powers, however, it is instrutive to
alulatethe limitabove whih this type of atomatom interation beomes signiant.
In dense samples of old atoms, two-atomproesses strongly inuene the trapping.
For example, ollisional proesses (photo-assoiation, hyperne ground state hanging
ollisions)are known toresultintraplosses andthey an limitthe maximumahievable
density. Collisions usually depend heavily on the internal eletroni struture of the
speies.Forinteratomidistanes intherange ofthe optialwavelength, the atom-atom
interation is dominatedby the radiativeeletromagneti oupling. In this ase one an
distinguish two limits: the photon sattering is dominated (i)by spontaneous emission,
e.g. in magneto-optial traps (MOT), and (ii) by stimulated emission, whih ours in
far-o-resonant dipoletraps (FORT). Sine the MOT enabled us rst toapture dense
atom louds from vapour, it was rst analyzed with respet to radiative many-body
eets [23, 140℄. In a MOT, the ooling laser is quasi-resonant with the atoms and the
sampleformsanoptiallythik medium.The depletionof thelaser beamstogether with
the multiple spontaneous sattering of resonant photons within the sample an lead to
instability[23℄andextraheating[141,142℄.Athighdensities,thereabsorptionofphotons
ina highlynonlinear olletivedynamis of the atom loud ina MOT [145, 146℄.
TheFORToperatesatanextremelylowspontaneoussatteringrate,thustheeets
of multiple spontaneous photon sattering are strongly suppressed. The mehanism of
trappingreliesontheproessofabsorptionandstimulatedemissionoflaserphotons.This
proesspolarizesthepartiles,henethedipoleforeisaompaniedbythedipole-dipole
ouplingbetweenatoms.Inpreviousworksaphenomenologialtermproportionaltothe
square of the atom density was introdued to desribe the atom-atom interation, e.g.,
the eet of ollisions on the loading of a FORT [147, 148℄. This dominates in strongly
loalized traps,ollisionalblokade an prevent us fromonning even twoatoms in an
extremely tiny FORT[149℄.
High atom densities an be an issue for many kinds of experiments with FORT's.
One example is the attempt to ahieve Bose-Einsteinondensation with alkali gases in
optial rather than magneti traps [150, 151℄. The stability of an atom loud against
dipole-dipole oupling is an issue also in the ultraold temperature regime where the
atoms forma degenerate Bose-ondensate. The orresponding anisotropi potentialan
beinludedintheGross-Pitaevkiequation[152℄.Thereisastablesolutionfortheatomi
mean-eld wavefuntion depending on the trap aspet ratio [153℄, or on the sattering
length [154, 155℄. The dipole-dipoleinteration gives rise to density modulations[156℄,
solitons [157℄. In these works the atoms possess a permanent dipolemoment. Reently,
the eets of the magneti dipole-dipole oupling has been observed in a hromium
ondensate[158℄.Thelaser indueddipole-dipoleouplingatlowtemperatureshas been
treatedin [159℄ and was shown tolead to nonlinear atom optial eets. An interesting
question arises that whether the dipole-dipole interation exludes the possibility of
forming aBose-Einstein ondensatein anoptial dipoletrap.
6.1 Dipole-dipole interation
The theory of radiative atom-atom interation in the presene of a driving laser eld
is desribed in several papers, e.g. Refs. [144, 159, 160, 161℄, we will mostly use the
approahpresented in [161℄.
Weonsider anumber
N
of atoms interating with a single Gaussianstanding-wave laser eld mode along thez ˆ
diretionwhihhas amode funtionf (r) = ǫ cos(k L z) exp
− 2π 2 (x 2 + y 2 )/w 2
,
(6.1)where
ǫ
is the eld polarization, and the mode is paraxial,k L ≫ 2π/w
. The atomitransition frequeny is
ω A
, that of the laser eld mode isω L
, and the detuning isde-ned by
∆ A = ω L − ω A
. The atom-mode interation strength is desribed by the Rabifrequeny
Ω
inthe positionofmaximum oupling.WeassumeanS ↔ P
transitionwitha degenerate manifold of exited states and keep the three-dimensional polarizability
of the atoms. Atually the xed eld polarization selets two levels taking part in the
dynamis. The atomi internal degree of freedom is desribed by the vetorial lowering
operator
σ = P
q ǫ q σ q
withq = ± 1
andq = 0
orresponding to the irular and linear polarizations, respetively. The quantizationaxis willbedened inaordane with thehoie of the eld polarization
ǫ
.The equation of motionfor the density operator inthe Markov approximationreads
˙ ρ = 1
i ~ [H, ρ] + L ρ .
(6.2)In aframe rotatingatthe laser frequeny
ω L
,the HamiltonianisH =
N
X
n=1
"
p 2
n
2m − ~ ∆ A σ † n σ n − i ~ Ω f (r n ) σ † n − σ n
#
− ~ γ
N
X
n,m=1 n 6 =m
σ † m β(R mn )σ n ,
(6.3)where
r n
,p
n
andσ n
are the position, the momentum and the polarization of then
thatom (
n = 1, . . . , N
).Next to the single atomterms, i.e.kineti energy, internal energy,and atom-eld oupling, the last term ontains the indued dipole-dipole interation
energyof theatoms. Notethatthe naturallinewidth
γ
haraterizesthe strength ofthis interation. The tensorβ
depends on the oordinate diereneR mn ≡ r m − r n
of theinterating pairs of atoms.
Thedipole-dipoleinteration ismediatedby thebroadbandvauum,and istherefore
aompanied by inoherent evolution. This is represented by additional terms in the
Liouvilleoperatorresponsible for the dissipation:
L ρ = − γ
N
X
n=1
{ σ † n σ n , ρ } − 2 X
q
Z
d 2 u N q (u)σ q n e − ik A ur n ρe ik A ur n σ n q †
− γ
N
X
n,m=1 n 6 =m
{ σ † m α(R mn )σ n , ρ } − 2 Z
d 2 u σ n N(u)e − ik A ur n ρe ik A ur m σ † m
,
(6.4)where
{ , }
denotes theantiommutator.Thesingleatomtermsinludethespontaneous deay aompanied by momentum reoil. The tensorN(u) = 3γ 8π (1 − u ◦ u)
, and itsdiagonal elements
N q (u) = ǫ q † N(u)ǫ q
are the angular momentum distribution of the spontaneousemissionfromtheq
-state inthe exited manifold.Here1
is thetwo-by-twounitmatrix, and
◦
denotes dyadi produt.The doublesumdesribesthelosseet duetothe dipole-dipoleoupling.
In free spae the tensors
α
andβ
assume the followingform :α(R mn ) = 3 2
(
(1 − R ˆ mn ◦ R ˆ mn ) sin kR mn
kR mn
+ (1 − 3 ˆ R mn ◦ R ˆ mn ) cos kR mn
(kR mn ) 2 − sin kR mn
(kR mn ) 3
!)
,
(6.5)β(R mn ) = 3 2
(
(1 − R ˆ mn ◦ R ˆ mn ) cos kR mn
kR mn
− (1 − 3 ˆ R mn ◦ R ˆ mn ) sin kR mn
(kR mn ) 2 + cos kR mn
(kR mn ) 3
!)
,
(6.6)where
k = | k | ≈ k L
,R mn = | R mn |
,andR ˆ mn
is a unit vetor along the diretion ofR mn
.The xed eld polarizationselets the exited state and the atom redues toa
two-level system with
σ n = σ n ǫ
(n = 1, . . . , N
). The tensorsα
andβ
have to be projetedontothis partiular polarization,
σ † m β(R mn )σ n = β(R mn )σ m † σ n ,
(6.7)where
β(R mn ) = ǫ † β(R mn )ǫ
. We now evaluate this projetion in two ases: for linearpolarizationalong
x ˆ
,and for irular one inthex ˆ
y ˆ
plane.6.1.1 Linear polarization
When the polarization of the beam is linear,
ǫ = ˆ x
, the atomi quantization axis is taken inthis diretion. Theatomi polarizationisdesribed by theoperatorσ 0
,and theprojetion given inEq. (6.7)results in
β mn = 3
2 (3 cos 2 φ mn − 1)
"
sin kR mn
(kR mn ) 2 + cos kR mn
(kR mn ) 3
# + 3
2 (1 − cos 2 φ mn ) cos kR mn
kR mn
,
(6.8)where
φ mn = ∡(R mn , x) ˆ
is the angle between the distane vetor of the two atoms andtheaxisof thepolarization,
x ˆ
.Asthis funtionissingularatthe origin,kR mn → 0
,laterwe willuse rather itsFourier transform [162℄,
β(k) = lim ˜
η → 0
√ 3 2πk L 3
(k z 2 + k 2 y ) (k 2 − k 2 L + η 2 )
(k 2 − k 2 L ) 2 + 2η 2 (k 2 + k L 2 ) .
(6.9)6.1.2 Cirular polarization
Ifthe polarizationisirular,
ǫ = − √ 1 2 (ˆ x + i y) ˆ
, the atomiquantizationaxis is the eld propagation diretionz ˆ
. The atomi polarizationis desribed by the operatorσ +1
, andthe projetion Eq. (6.7) gives
β mn = 3
4 (1 − 3 cos 2 θ mn )
"
sin kR mn
(kR mn ) 2 + cos kR mn
(kR mn ) 3
# + 3
4 (cos 2 θ mn + 1) cos kR mn
kR mn
.
(6.10)The angle
θ mn = ∡(R mn , z) ˆ
is the angle between the distane vetor of the two atomsand the axis